外源对太湖河口沉积物有机质贡献的同位素示踪

曾海鳌, 吴敬禄

曾海鳌, 吴敬禄. 外源对太湖河口沉积物有机质贡献的同位素示踪[J]. 海洋地质与第四纪地质, 2009, 29(1): 109-114. DOI: 10.3724/SP.J.1140.2009.01109
引用本文: 曾海鳌, 吴敬禄. 外源对太湖河口沉积物有机质贡献的同位素示踪[J]. 海洋地质与第四纪地质, 2009, 29(1): 109-114. DOI: 10.3724/SP.J.1140.2009.01109
ZENG Haiao, WU Jinglu. ISOTOPIC TRACING OF TERRESTRIAL CONTRIBUTION TO ORGANIC MATTER OF SEDIMENTS IN THE ESTUARY OF TAIHU LAKE BASIN[J]. Marine Geology & Quaternary Geology, 2009, 29(1): 109-114. DOI: 10.3724/SP.J.1140.2009.01109
Citation: ZENG Haiao, WU Jinglu. ISOTOPIC TRACING OF TERRESTRIAL CONTRIBUTION TO ORGANIC MATTER OF SEDIMENTS IN THE ESTUARY OF TAIHU LAKE BASIN[J]. Marine Geology & Quaternary Geology, 2009, 29(1): 109-114. DOI: 10.3724/SP.J.1140.2009.01109

外源对太湖河口沉积物有机质贡献的同位素示踪

基金项目: 

国家自然科学基金项目(40673015)

中科院知识创新工程项目(KZCX2-YW-319)

详细信息
    作者简介:

    曾海鳌(1980-),男,助理研究员,从事环境地球化学研究,E-mail:zenghaiao@niglas.ac.cn

  • 中图分类号: P593

ISOTOPIC TRACING OF TERRESTRIAL CONTRIBUTION TO ORGANIC MATTER OF SEDIMENTS IN THE ESTUARY OF TAIHU LAKE BASIN

  • 摘要: 分析了太湖流域不同土地利用类型土壤、河口表层沉积物及主要生物的有机碳含量和同位素分布特征,并利用端元混合法求取了陆源输入对湖泊沉积物有机质的贡献及分布。研究结果表明,流域表层土壤有机质δ13C受植物群落的δ13C值影响,不同植被类型的土壤有机质δ13C值存在差异。茶园、菜地、林地和农田δ13Corg平均值分别为-25.4‰、-25.8‰、-27.1‰和-28.1‰,其中茶园有机碳同位素值最高。河口表层沉积物有机碳同位素变化范围为-27.5‰~-25.1‰,平均值为-25.7‰。河口近岸区域表层沉积物δ13Corg偏低,且以河口为轴心向湖心逐渐增大,呈扇形条状分布,其分布主要受低δ13C值的陆源有机质输入影响。利用端元混合法求得近河口表层沉积物中陆源有机质贡献高达70%~80%,随着离岸距离的增加,陆源有机质贡献量逐渐减少。
    Abstract: The authors analyzed characteristics of organic carbon content and isotope distribution of top soil in different Land use types within the Taihu Lake basin, as well as surface sediments and organisms within the estuary. The sources of organic matter of lake sediments were obtained by using two-member mixing model. The results showed that there were differences of organic δ13C in different plant types, which affected organic δ13C of top soil within the catchment. The average δ13Corg values of tea plantations, vegetable lands, forest lands and paddy fields were -25.4‰,-25.8‰,-27.1‰ and -28.1‰ respectively,and the highest δ13Corg value existed in tea plantations. The range of δ13Corg values of surface sediments within the estuary were -27.5‰~-25.1‰ with the average value of -25.7‰. The δ13Corg of surface sediments near the shore was low, and gradually decreased from the estuary to center. The reason was the effect of import of terrestrial source with lower δ13Corg values. By using two-member mixing model, the contribution ratios of terrestrial source was 70%~80% in the estuary, and gradually decreased with the distance to the lake shore.
  • [1] 黄漪平.太湖水环境及其污染控制[M]. 北京:科学出版社,2001:1-53.[HUANG Yipins. The Water Environment and Pollution Control of Taihu Lake[M]. Beijing:Science Press,2001:1

    -53]

    [2] 秦伯强,范成新. 大型浅水湖泊内源营养盐释放的概念性模式探讨[J]. 中国环境科学,2002,22(2):150-153.

    [QIN Boqing,FAN Chengxin. Exploration of conceptual model of nutrient release from inner source in large shallow lake[J]. China Environmental Science,2002,22(2):150-153]

    [3]

    Wu J L,Huang C M,Zeng H A,et al. Sedimentary evidence for recent europhication in the northern basin of lake Taihu, China:human impacts on a large shallow lake[J]. Journal of Paleolimnology,2007,38(1):13-23]

    [4]

    Hopkinson C S,Buffam I,Hobbie J,et al. Terrestrial inputs of organic matter to coastal ecosystems:an intercomparison of chemical characteristics and bioavailability[J]. Biogeochemistry,1998,43,211-234.

    [5]

    Raymond P A,Bauer J E. Bacterial consumption of DOC during transport through a temperate estuary[J]. Aquatic Microbial Ecology,2000,22:1-12.

    [6]

    D'Angelo E M,Reddy K R. Diagenesis of organic matter in a wetland receiving hypereutrophic lake water:I. Distribution of dissolved nutrients in the soil and water column[J]. Journal of Environmental Quality, 1994,23(5):928-936.

    [7]

    Peterson B J. Stable isotopes as tracers of organic matter input and transfer in benthic food webs:a review[J]. Acta Oceanologica Sinica,1999,20(4):479-487.

    [8]

    Cloern J E,Canuel E A,Harris D. Stable carbon and nitrogen isotope composition of aquatic and terrestrial plants of the San Francisco Bay estuarine system[J]. Limnology and Oceanography,2002,47(3):713-729.

    [9]

    Andrews J E,G reenaway A M,Dennis P F. Combined carbon isotope and C/N ratios as indictors of source and fate of organic matter in a poorly flushed,tropical estuary[J]. Coastal and Shelf Science,1998,46:743-756.

    [10]

    Graham M C. A study of carbon and nitrogen stable isotope and elemental ratios as potential indicators of source and fate of organic matter in sediments of the Forth Estuary, Scotland[J]. Estuarine,Coastal and Shelf Science,2001,52:375-380.

    [11]

    Goñi M A,Maria J T,Perkey D W. Sources and distribution of organic matter in a river-dominated estuary (Winyah Bay,SC,USA)[J]. Estuarine,Coastal and Shelf Science,2003,57:1023-1048.

    [12]

    Vaalgamaa S,Conley D J. Detecting environmental change in estuaries:Nutrient and heavy metal distributions in sediment cores in estuaries from the Gulf of Finland, Baltic Sea[J]. Estuarine,Coastal and Shelf Science,2008,76(1):45-56.

    [13]

    Wu Y,Zhang J,Li D J,et al. Isotope variability of particulate organic matter at the PN section in the East China Sea[J]. Biogeochemistry,2003,65(1):31-49.

    [14] 史云祥. 宜深河流域水环境演变趋势以及污染物输移过程研究[D]. 南京理工大学硕士学位论文,2002.[SHI Yunxiang.The study of the water environmental change trend and contaminant transportation in Yili river basin[D]. Master Dissertation of Nanjing University of Science and Technology,2002]
    [15] 曾庆飞,孔繁翔,张恩楼,等. 利用稳定同位素技术研究外源物质输入对太湖微食物链的贡献[J]. 环境科学,2007,28(8):1670-1673.

    [ZENG Qingfei,KONG Fanxiang,ZHANG Enlou,et al. Effects of anthropogenic organic matter inputs on stable carbon and nitrogen isotopes in organisms from microbial food chain in Taihu Lake[J]. Environment Science,2007,28(8):1670-1673]

    [16] 高建华,汪亚平,潘少明,等. 长江口外海域沉积物中有机物的来源及分布[J]. 地理学报, 2007,62(9):81-91.

    [GAO Jianhua,WANG Yaping,PAN Shaoming,et al. Source and distribution of organic matter in seabed sediments of the Changjiang River estuary and its adjacent sea area[J]. Acta Geographic Sinica,2007,62(9):81-91]

    [17]

    Mayer L M. Surface area control of organic carbon accumulation in the continental shelf sediments[J]. Geochemica et Cosmochimica Acta,1994,58(4):1271-1284.

    [18]

    Keil R G,Tsamakis E C,Fuh C B,et al. Mineralogical and texture controls on the organic composition of coastal marine sediments[J]. Geochemica et Cosmochimica Acta,1994,58(2):879-893.

    [19]

    Staddon P L. Carbon isotopes in functional soil ecology[J]. Trends in Ecology and Evolution,2004,19(3):148-154.

    [20] 李志鹏,潘根兴,张旭辉. 改种玉米连续3年后稻田土壤有机碳分布和13C自然丰度变化[J]. 土壤学报,2007,44(2):244-251.

    [LI Zhipeng,PAN Genxing,ZHANG Xuhui. Topsoil organic carbon pool and 13C natural abundance changes from a paddy after 3 years corn cultivation[J]. Acta Pedologica Sinica,2007,44(2):244-251.]

    [20]

    Schweizer M,Fear J,Cadisch G. Isotopic (13C) fractionation during plant residue decomposition and its implications for soil organic matter studies[J]. Rapid Communications in Mass Spectrometry,1999,13:1284-1290.

    [21] 曾海鳌,吴敬禄,林琳. 137Cs示踪法研究太湖流域土壤侵蚀分布与总量[J]. 海洋地质与第四纪地质, 2008, 28(2):79-85.

    [ZENG Haiao,WU Jinglu,LIN Lin. Using 137Cs tracer technique to investigate the soil erosion distribution and total erosion amount in Taihu Lake catchment[J]. Marine Geology and Quaternary Geology,2008,28(2):79-85]

计量
  • 文章访问数:  1910
  • HTML全文浏览量:  273
  • PDF下载量:  16
  • 被引次数: 0
出版历程
  • 收稿日期:  2008-10-26
  • 修回日期:  2009-01-05

目录

    /

    返回文章
    返回